PokéBase - Pokémon Q&A
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Anything ranging from NPCs who need help to NPCs who just want to see Pokemon.

I'd also like where the NPCs are, what Pokemon they need, and if possible, how I can receive those Pokemon.

Thanks!

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My eye twitched just then.
Don't worry.
There's a lot more where that came from. ;)
Oh no not again
Heart Sclae- Drifveil city (If you show a girl the move she requests)

Soothe Bell – Nimbasa City (show a Pokemon with high Happiness to NPC in building north of Battle Institute)
This is what i found for now.

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Accumula Town

Poké Doll - From a Youngster after showing him a Pokémon that is 8" (20 cm) or smaller (once per day)
Fluffy Tail - From a Lass after showing her a Pokémon that is 17' (5 m) or bigger (once per day)
Metronome - From the pianist in the northeastern house after showing her a Kricketot and a Whismur

Straiton City

Gracidea - Gift from the girl inside the Pokémon Center if she is shown a fateful encounter Shaymin.

Driftveil City

Heart Scale - From a woman in the house south of the market, if the player has a Pokémon knowing the asked TM move (repeatable once per day)
Expert Belt - Received from a man in black at the market, if the player has a Pokémon that is level 30 or higher

Mistralton City

Net Ball x5 - Pilot behind the counter in the Cargo Service building, for bringing him a Flying- or Psychic-type Pokémon

Icirrus City

Exp. Share - Gift from chairman of the Pokémon Fan Club, if Pokémon shown has gained between 25 and 49 levels since it was met in a Generation V game
Cleanse Tag - Gift from chairman of the Pokémon Fan Club, if Pokémon shown has gained between 50 and 98 levels since it was met in a Generation V game
King's Rock - Gift from chairman of the Pokémon Fan Club, if Pokémon shown has gained 99 levels since it was met in a Generation V game

P2 Laboratory

Shock/Burn/Douse/Chill Drive - Show Genesect to Scientist Dudley inside (Given drive(s) will vary depending on version)

Abundant Shrine

Reveal Glass - Obtained from a man near Landorus's shrine if a Therian Forme Landorus is brought there

Marine Tube

Black Sludge - After showing an NPC a Pokémon holding a Poison Barb

Route 2

Dawn Stone - Gift from a Lady east of Youngster Mikey for showing her a Pokémon with Solid Rock.

Route 4

Swift Wing ×1 or ×5 - From male Ace Trainer in a house near Lady Lina if he is shown a Pokémon with an Attack stat equal to (gives five) or higher (gives one) than what he requests. Can be repeated daily, with request values changing every time.

Gone through all the places, routes and cites. can't find more. Also, Arcazeus's Soothe Bell one apparently only applies to BW not B2W2 (Checked on Bulbapedia)

Also I didn't include people who want to trade with you/people who give you items after you have seen a certain amount of Pokemon, rather than a specific Pokemon.

Anyone feel free to comment any I forgot, and I'll double check it

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There's one more in south Unova, a lass who was asking to see a pokemon with Solid Rock too I think
Can't find it.
On a route if I'm right, lemme try looking for it
Lady on Route 2 wants to see a pokemon with Solid Rock. She gives you a Dawn Stone if you do.
I already have that. Read my answer
Dawn Stone - Gift from a Lady east of Youngster Mikey for showing her a Pokémon with Solid Rock.
Oh. [filler]