One option is a Quick Ball - an awesome quick alternative to expensive Ultra Balls. They work on 80% of Pokemon, and probably not legendaries. If you mean Raikou, or another wandereing Pokemon, Kepp hacking away with False Swipe until it has 1 Hp. Then try to put it to sleep, or paralyze it. Finally, throw a Quick Ball, a heavy Ball for Raikou or Entei, and maybe Dusk Balls if it's night. It helps to have a Pokemon like Chandelure so it won't flee.