PokéBase - Pokémon Q&A
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It seems that every time I try to catch primal kyogre, all of my pokeballs don't work so is ultra ball the best the catch the Pokemon.

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Ultra balls are always better than pokeballs and great balls. Though Dusk balls would also work well, since you're in a cave while catching Kyogre. I would also recommend having a quick ball, which works very well on the first turn.

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