PokéBase - Pokémon Q&A
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Can you use any type pokeball? Also, where do yo find Zekrom?

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1 Answer

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A. Yes, he was ridiculously easy for me to catch, I caught him first try with a Great Ball.

B. You find him in N's Castle shortly after you defeat the Elite Four.

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I caught him with a regular pokeball.
My sister caught Reshiram with a great ball... I accidently used my master ball on a pokemon that was easy to catch....
I caught Reshiram in a Quick Ball on the first turn.  It's fun to use those :)