PokéBase - Pokémon Q&A
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>All Pokémon that can learn TMs can learn Substitute. -Bulbepedia

These Pokemon can't learn any TMs:

  • Caterpie

  • Metapod

  • Weedle

  • Kakuna

  • Magikarp

  • Ditto

  • Unown

  • Wobbuffet

  • Smeargle

  • Wurmple

  • Silcoon

  • Cascoon

  • Wynaut

  • Beldum

  • Kricketot

  • Burmy

  • Combee

  • Tynamo

Source^

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Why can't Tynamo learn TMs?
I dunno lol