PokéBase - Pokémon Q&A
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They are held by wild pikachu with a 5% chance so keep catching pikachus in the trophy garden or have a frisk Pokemon to see if it holds a light ball and then you will find a pikachu holding one eventually.
Source: http://bulbapedia.bulbagarden.net/wiki/Light_ball#Light_Ball

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The Pikachus in Mr. Backlot's Trophy Garden have a 5% chance of holding a Light Ball.

Source: Experience

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On Route 202 I believe the route with the Trophy Garden Mansion. There is a 5% chance a wild Pikachu will hold a Light Ball. A Pokemon with the ability Frisk is helpful so you don't capture/ steal from the wrong Pikachu.

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