Meta Rate My Team PokéBase - Pokémon Q&A
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zekrom is easier to catch because it has a higher catch rate at 45 while kyurem has a catch rate of 3.
Source:
http://bulbapedia.bulbagarden.net/wiki/Kyurem
http://bulbapedia.bulbagarden.net/wiki/Zekrom

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in white and black i throw 1 ultra ball to zekrom and reshiram and i captured them :]