PokéBase - Pokémon Q&A
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You must sneak up to them using the DexNav. They're those Pokémon with part of their body sticking out of the grass and you must gently push the Circle Pad to sneak up to them.

Source: http://pokemondb.net/location/hoenn-jagged-pass

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Of course, you need the National Pokédex, but you already have it.