PokéBase - Pokémon Q&A
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In crystal, you can catch Lugia (whirl islands), Ho-oh (tin tower), Suicune (is encountered throughout the game, but is ultimately battled in one of the towers in Ecruteak city), and last but not least, Raikou/Entei (roaming throughout the game.)

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Lugia is in the whirl islands.
Ho oh is in the tin tower.
Suicune wanders around all over the place, but eventually stops.

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